As global industrialization leads to an increase in atmospheric CO₂ concentration, causing environmental issues, reducing CO₂ emissions has become a consensus. CO₂mineralization storage technology has garnered attention, with ultrabasic tailings being ideal raw materials due to their rich content of magnesium, iron, and other elements. This study centers on the carbonation of ultrabasic tailings, investigating its kinetic mechanisms and optimizing conditions. The research framework encompasses the kinetics of direct aqueous carbonation of olivine under a CO₂ partial pressure of 6.5 MPa, the mechanism of mechanical activation of multiphase ultrabasic tailings, and the feasibility study of ultrabasic mine exploitation in conjunction with CO₂ mineralization storage technology. In terms of research methods, olivine from Washington State, USA, and tailings from northern British Columbia, Canada, were selected as materials. Experiments were carried out using a stirred autoclave manufactured by Parr Instrument Company (USA), with additional equipment such as a laser diffraction particle size analyzer employed for characterization purposes. Quantitative analysis of product composition and chemical kinetic theory were used to analyze the reaction. The research results show that optimizing conditions under low CO₂ partial pressure can significantly enhance the degree of olivine carbonation, and mechanical activation can increase the reactivity of minerals, providing theoretical support for the promotion of ultrabasic mine exploitation in conjunction with CO₂ mineralization storage technology
Research Article
Open Access